1. osnaDocs
  2. Fachbereich 06 - Mathematik / Informatik / Physik
  3. FB06 - Hochschulschriften

Atomic insight to lattice distortions caused by carrier self-trapping in oxide materials

Please use this identifier to cite or link to this item:
https://osnadocs.ub.uni-osnabrueck.de/handle/urn:nbn:de:gbv:700-2017032715706
Open Access logo originally created by the Public Library of Science (PLoS)
Full metadata record
DC FieldValueLanguage
dc.creatorFreytag, Felix
dc.creatorCorradi, Gábor
dc.creatorImlau, Mirco
dc.date.accessioned2017-03-27T06:52:04Z
dc.date.available2017-03-27T06:52:04Z
dc.date.issued2017-03-27T06:52:04Z
dc.identifier.citationScientific Reports, Vol. 6; Article number: 36929, 2016, S. 1-7
dc.identifier.urihttps://osnadocs.ub.uni-osnabrueck.de/handle/urn:nbn:de:gbv:700-2017032715706-
dc.description.abstractWe gain hitherto missing access to the spatio-temporal evolution of lattice distortions caused by carrier self-trapping in the class of oxide materials - and beyond. The joint experimental/theoretical tool introduced combines femtosecond mid-infrared probe spectroscopy with potential landscape modeling and is based on the original approach that the vibration mode of a biatomic molecule is capable to probe strongly localized, short-lived lattice distortions in its neighborhood. Optically generated, small, strong-coupling polarons in lithium niobate, mediated by OH− ions present as ubiquitous impurities, serve as a prominent example. Polaron trapping is found to result in an experimentally determined redshift of the OH− stretching mode amounting to Δνvib = −3 cm−1, that is successfully modeled by a static Morse potential modified by Coulomb potential changes due to the displacements of the surrounding ions and the trapped charge carrier. The evolution of the trapping process can also be highlighted by monitoring the dynamics of the vibrational shift making the method an important tool for studying various systems and applications.
dc.relationhttp://www.nature.com/articles/srep36929
dc.rightsNamensnennung 4.0 International-
dc.rights.urihttp://creativecommons.org/licenses/by/4.0/-
dc.subjectInfrared spectroscopyeng
dc.subjectNonlinear opticseng
dc.subjectUltrafast photonicseng
dc.subject.ddc530 - Physik
dc.titleAtomic insight to lattice distortions caused by carrier self-trapping in oxide materialseng
dc.typeEinzelbeitrag in einer wissenschaftlichen Zeitschrift [article]
dc.identifier.doi10.1038/srep36929
vCard.ORGFB4
Appears in Collections:FB06 - Hochschulschriften
Open-Access-Publikationsfonds

Files in This Item:
File Description SizeFormat 
Zeitschriftenartikel_Scientific_Reports_6_36929_2016_Freytag_etal.pdf2,04 MBAdobe PDF
Zeitschriftenartikel_Scientific_Reports_6_36929_2016_Freytag_etal.pdf
Thumbnail
View/Open
Show simple item record


This item is licensed under a Creative Commons License Creative Commons